Noble metallic nanostructures with strong electric near-field enhancement can significantly improve nanoscale light–matter interactions and are critical for high-sensitivity surface-enhanced Raman spectroscopy (SERS). Here, we use an azimuthal vector beam (AVB) to illuminate the plasmonic tips circular cluster (PTCC) array to enhance the electric near-field intensity of the PTCC array, and then use it to improve SERS sensitivity. The PTCC array was prepared based on the self-assembled and inductive coupled plasmon (ICP) etching methods. The calculation results show that, compared with the linearly polarized beam (LPB) and radial vector beam excitations, the AVB excitation can obtain stronger electric near-field enhancement due to the strong resonant responses formed in the nanogap between adjacent plasmonic tips. Subsequently, our experimental results proved that AVB excitation increased SERS sensitivity to 10^-13 mol/L, which is two orders of magnitude higher than that of LPB excitation. Meanwhile, the PTCC array had excellent uniformity with the Raman enhancement factor calculated to be ∼2.4×108. This kind of vector light field enhancing Raman spectroscopy may be applied in the field of sensing technologies, such as the trace amount detection.

Cylindrical vector beams and vortex beams, two types of typical singular optical beams characterized by axially symmetric polarization and helical phase front, possess the unique focusing property and the ability of carrying orbital angular momentum. We discuss the formation mechanisms of such singular beams in few-mode fibers under the vortex basis and show recent advances in generating techniques that are mainly based on long-period fiber gratings, mode-selective couplers, offset-spliced fibers, and tapered fibers. The performances of cylindrical vector beams and vortex beams generated in fibers and fiber lasers are summarized and compared to give a comprehensive understanding of singular beams and to promote their practical applications.

We present the generation of the nanosecond cylindrical vector beams (CVBs) in a two-mode fiber (TMF) and its applications of stimulated Raman scattering. The nanosecond (1064 nm, 10 ns, 10 Hz) CVBs have been directly produced with mode conversion efficiency of ～18 dB (98.4%) via an acoustically induced fiber grating, and then the stimulated Raman scattering signal is generated based on the transmission of the nanosecond CVBs in a 100-m-long TMF. The transverse mode intensity and polarization distributions of the first-order Stokes shift component (1116.8 nm) are consistent with the nanosecond CVBs pump pulse.

Goodness of fit is demonstrated for theoretical calculation of z-scan data based on beams propagating in the nonlinear medium and the Fresnel–Kirchhoff diffraction integral in experiments with high nonlinear refraction and absorption. The constancy of nonlinear optical parameters is achieved regardless of sample thickness and laser intensity, which clarifies the physical significance of optical parameters. We have obtained γ = 2.0 × 10^?19 m²/W and β = 5.0 × 10^?13 m/W for carbon disulfide excited by a pulsed laser at 800 nm with pulse duration of 35 fs, which are independent of sample thickness and laser intensity. Affirming constancy of the extracted parameters to the incident light intensity may become a practice to verify the goodness of the z-scan experiment.

A polarization-insensitive plasmonic absorber is designed consisting of Au fishnet structures on a TiO₂ spacer/Ag mirror. The fishnet structures excite localized surface plasmon and generate hot electrons from the absorbed photons, while the TiO₂ layer induces Fabry–Perot resonance, and the Ag mirror acts as a back reflector. Through optimizing the TiO₂ layer thickness, numerical simulation shows that 97% of the incident light is absorbed in the Au layer. The maximum responsivity and external quantum efficiency of the device can approach 5 mA/W and ～1%, respectively, at the wavelength of 700 nm.

Surface-enhanced Raman spectroscopy (SERS) with high-sensitivity performance is a very necessary detection technology. Here, we present a method for increasing the performance of SERS based on silver triangular nanoprism arrays (ATNAs) vertically excited via a focused azimuthal vector beam (AVB). The ATNA substrates with different structural parameters are prepared based on the traditional self-assembled and modified film lift-off technique. Based on a theoretical model established adopting the structural parameters of the ATNA substrates, theoretical simulation results show that AVB excitation can achieve greater electric-field enhancement than linearly polarized beam (LPB) excitation. Experimental result indicates that SERS sensitivity obtained via AVB excitation is 10 13M (1 M = 1 mol/L) using rhodamine 6G (R6G) as the target analyte, which is 2 orders of magnitude lower than that of LPB excitation (10 11M). Meanwhile, the uniformity and reproducibility of the ATNA substrates are examined using Raman mapping and batch-to-batch measurement, respectively, and the Raman enhancement factor is calculated to be ～3.3×107. This method of vector light field excitation may be used to improve the SERS performance of the substrates in fields of ultra-sensitive Raman detection.

Acousto-optic interactions, employed in the ultrafast laser regulation, possess remarkable advantages for fast tuning performance in a wide spectral range. Here, we propose an ultrafast fiber laser whose wideband tunability is provided by an acousto-optic structure fabricated with an etched single-mode fiber. Because of the laser polarization conversion induced by the coupling between the core and cladding vector modes in the etched fiber, a band-pass characteristic of the acousto-optic interaction is achieved to effectively regulate the inner-cavity gain range. Cooperating with a saturable absorber based on single-wall carbon nanotubes (SWCNTs) with polarization robustness, a soliton operating state is achieved in the tunable erbium-doped fiber laser. By controlling the acoustical wave frequency from 1.039 to 1.069 MHz, this soliton laser can be conveniently tuned in a wide spectral range from 1571.52 to 1539.26 nm. Meanwhile, the laser pulses have near-transform-limited durations stably maintaining less than 2 ps at different wavelength channels, owing to the broadband nonlinear absorption of SWCNTs.

The synergy of a plasmonic tip and fiber-based structure light field excitation can provide a powerful tool for Raman examination. Here, we present a method of Raman spectrum enhancement with an Ag-nanoparticles (Ag-NPs)-coated fiber probe internally excited via an azimuthal vector beam (AVB), which is directly generated in a few-mode fiber by using an acoustically induced fiber grating. Theoretical analysis shows that gap mode can be effectively generated on the surface of the Ag-NPs-coated fiber probe excited via an AVB. The experimental result shows that the intensity of Raman signal obtained with analyte molecules of malachite green by exciting the Ag-NPs-coated fiber probe via an AVB is approximately eight times as strong as that via the linear polarization beam (LPB), and the activity of the AVB-excited fiber probe can reach 10 11 mol/L, which cannot be achieved by LPB excitation. Moreover, the time stability and reliability are also examined, respectively.

Plasmon induced hot electrons have attracted a great deal of interest as a novel route for photodetection and light-energy harvesting. Herein, we report a hot electron photodetector in which a large array of nanocones deposited sequentially with aluminum, titanium dioxide, and gold films can be integrated functionally with nanophotonics and microelectronics. The device exhibits a strong photoelectric response at around 620 nm with a responsivity of 180 μA/W under short-circuit conditions with a significant increase under 1 V reverse bias to 360 μA/W. The increase in responsivity and a red shift in the peak value with increasing bias voltage indicate that the bias causes an increase in the hot electron tunneling effect. Our approach will be advantageous for the implementation of the proposed architecture on a vast variety of integrated optoelectronic devices.